An investigation of the effect of pore scale flow on average geochemical reaction rates using direct numerical simulation

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An investigation of the effect of pore scale flow on average geochemical reaction rates using direct numerical simulation

The scale-dependence of geochemical reaction rates hinders their use in continuum scale models intended for the interpretation and prediction of chemical fate and transport in subsurface environments such as those considered for geologic sequestration of CO2. Processes that take place at the pore scale, especially those involving mass transport limitations to reactive surfaces, may contribute t...

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ژورنال

عنوان ژورنال: Water Resources Research

سال: 2012

ISSN: 0043-1397

DOI: 10.1029/2011wr011404